Baudoin Research Group
@Baudoin_Group
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Student-run account for the Baudoin Group at @UniBasel
Joined February 2021
We are happy to share that from now on we'll be posting exciting news from our group on Bluesky! 🧪 Same research 🧪 Same passion for catalysis and C-H activations 🧪 New platform! https://t.co/2fSN9RYz8g Follow us on Bluesky to stay updated on our latest work!
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Exciting news from the 7th International Symposium on C-H Activations in Mumbai @ischa2024 ! Olivier delivered an inspiring lecture on direct Pd-catalyzed ring construction via C(sp3)–H activation. 🧪It was a pleasure and a great experience! #CHActivation #Chemistry
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Exciting days for the Baudoin Group! 🎓 Maria & Andrea successfully defended their PhDs, making significant contributions to Pd, Ir, and Fe-catalyzed C-H functionalizations. Huge congrats to both, and best wishes for the future! 🚀👏 #BaudoinGroup #PhD #Chemistry #PhDone
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Fe-Catalyzed alpha-C(sp3)-H Amination of N-Heterocycles (Olivier Baudoin and co-workers) @Baudoin_Group @UniBasel_en #openaccess
onlinelibrary.wiley.com
An iron(II)-catalyzed α-selective C−H amination of N-heterocycles is reported. It employs the N-heterocycle as the limiting reagent and presumably involves the formation of a reactive Fe-nitrene/im...
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The list of most accessed papers in October includes contributions by @Baudoin_Group, @subohxx, @alexanderln91 - what else? https://t.co/LgLy0gcAeo
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Interested in C-H amination of pharmaceutically relevant motifs? You can use just FeCl2 as a catalyst for that. Our paper on Fe-catalyzed C(sp3)-H amination was published in Angewandte @angew_chem. Check it out here: https://t.co/qekNYWEKmt
#catalysis #Chemistry #amination
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Pierre and Kseniia have joined our research group for their PhD studies! We are excited to have them on board and wish them a lot of success in their future projects!
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Oleks just won the runner-up prize for the oral presentation of our recent total syntheses of Randainin D and Barekoxide at the SCS Fall Meeting 2024 in the Organic Chemistry section. Congrats Oleks! #OrganicSynthesis #SCS #FallMeeting @SwissChemistry
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Can you complete the forward synthesis of (+)-Randainin D without seeing its structure? On the last #LCSOSynthesisProblem Christine challenged us with its synthesis by @Baudoin_Group in @J_A_C_S. Take a look: https://t.co/a4xph9gS8P Original paper:
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Wonderful talk on palladium catalyzed C-H activation leading to complex fused ring systems. by @Baudoin_Group, the 2024 plenary lecturer @LIMA_UMR7042 spring day.
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Plenary lecture by @Baudoin_Group on palladium catalyzed construction of fused ring systems. @LIMA_UMR7042 spring day 2024
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Interested in cyclobutanes, azetidines and oxetanes?🔳 Check out our just-published paper on the synthesis of fused 4-membered rings enabled by 1,4-palladium migration! @J_A_C_S Read more here: https://t.co/7IklkN5pks
1,4-Pd Migration-Enabled Synthesis of Fused 4-Membered Rings | Journal of the American Chemical Society @Baudoin_Group @UniBasel @TotalSyntheses #Pd #Migration #Benzocycloalkenes #Bicyclooctenes
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New approaches to #terpene synthesis: Researchers at @UniBasel_en present an innovative approach to producing these versatile natural substances, including those already used in #therapies for cancer, epilepsy, and malaria. https://t.co/y0SjDZoGYd
unibas.ch
They are found as fragrances in cosmetics or as flavorings in food, and form the basis of new medications: Terpenes are natural substances that occur in plants, insects and sea sponges. They are...
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Synthesis of the Diterpenes (+)-Randainin D and (+)-Barekoxide via Photoredox-Catalyzed Deoxygenative Allylation | JACS @Baudoin_Group @UniBasel @TotalSynthesis @TotalSyntheses #Diterpene #Photoredox #Allylation
pubs.acs.org
We report the first enantioselective total synthesis of diterpenoid randainin D, which possesses a hydroazulenone core with a β-substituted butenolide moiety on the cycloheptane ring. The trans-5/7...
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Our total synthesis of (+)-randainin D and (+)-barekoxide via photoredox-catalyzed deoxygenative allylation is now out in @J_A_C_S. You can find the article here: https://t.co/9QSpsjrC8z
#TotalSynthesis
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Our work on the studies towards the total synthesis of cryptowolinol is now out in @JOC_OL. The key step is a challenging enantioselective Pd0-catalyzed C(sp3)–H arylation, which proceeds via PKR. You can read more about it here: https://t.co/4TvTq3vTlV
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Methylene C(sp3)-H Arylation Enables the Stereoselective Synthesis and Structure Revision of Indidene Natural Products (Olivier Baudoin and co-workers) @Baudoin_Group
onlinelibrary.wiley.com
The indane polyketides indidenes A and C were synthesized from a common intermediate through nickel-catalyzed dehydrogenative coupling and Suzuki–Miyaura coupling, respectively. The common diol...
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Our work on the total synthesis of indidene natural products has been accepted in @angew_chem. To find out more about the methylene C(sp3)–H activation and structure revisions, you can read the article here: https://t.co/HPhj87xmFr
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We are currently looking for high-profile chemists to apply to SNSF Swiss Post-doctoral Fellowships. Please check our website for all details:
baudoin.chemie.unibas.ch
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Our mechanistic studies on the effect of α-substitution on the reactivity of Pd-catalyzed C(sp3)–H activation has been accepted in @ACSCatalysis. You can read the paper here: https://t.co/sE3JJCqDLi
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